FireWire 800's sub-100MB/s speeds will probably still be unsatisfactory, given that single 7200rpm spindles run at 150MB/s these days, and your desire to fast transfer speeds.
In other words, I'd spend the money on a native TB storage device - Promise or G-Tech. R4 will likely be faster, and offers better use of space with RAID5 redundancy, vs. RAID1.
Alex Gerulaitis
Systems Integrator
DV411 - Los Angeles, CA